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Laboratory of Physical Chemistry and optETH, ETH Zürich Quantum Optics with Single Molecules In this seminar I shall discuss several experimental and theoretical investigations of coupling strength between propagating light beams and single emitters. We show that a single dye molecule can strongly attenuate a laser beam and discuss the conditions for reaching this fascinating regime [1-3]. We find that such an efficient light-matter coupling allows several nonlinear processes to be achieved at low photon levels and present experimental results on the observation of single-molecule Rabi oscillations [4] and stimulated emission from a single molecule which can act as an optical transistor [5]. In the last part of the talk, I shall present our recent progress on the coupling of two molecules at large distances, the preparation of indistinguishable photons from independent sources [6], and the demonstration of the Hong-Ou-Mandel two-photon interference of single photons [7]. [1] G. Zumofen, N.M. Mojarad, V. Sandoghdar, and M. Agio, Phys. Rev. Lett. 101, 180404 (2008). |